Publikation: Dissertationsschrift

Laser-driven electron and spin-state quantum dynamics in transition metal complexes

Grunddaten
Abstract
Autoren
Einrichtung

Grunddaten

Titel	Laser-driven electron and spin-state quantum dynamics in transition metal complexes
Erscheinungsjahr	2018
Verlag	Universität Rostock
Verlagsort	Rostock
Seitenzahl	98
Publikationsform	Druckschrift
Publikationsart	Dissertationsschrift
Sprache	Englisch
Letzte Änderung	14.05.2019 10:28:56
Bearbeitungsstatus	durch UB Rostock abschließend validiert
Dauerhafte URL	http://purl.uni-rostock.de/fodb/pub/59364
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Abstract

Recent advances in attosecond spectroscopy open the door to the understanding correlated motion of valence and core electrons in molecular systems. In this thesis, the density matrix-based TD-RASCI method is used to study the electron and spin-flip dynamics. The dephasing effect of nuclear vibrations is incorporated implicitly making use of an electronic system/vibrational bath partitioning. We theoretically addressed the ultrafast spin-flip dynamics in a transition metal complex which is triggered by isolated sub-fs soft-X-ray pulses as well as X-ray pulse trains.

Autor

Wang, Huihui

Einrichtung

MNF/Institut für Physik (IfPH)